Artículo

El editor no permite incluir ninguna versión del artículo en el Repositorio.
Consulte el artículo en la página del editor
Consulte la política de Acceso Abierto del editor

Abstract:

Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit. © 2011 Optical Society of America.

Registro:

Documento: Artículo
Título:Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
Autor:Brinks, D.; Hildner, R.; Stefani, F.D.; Van Hulst, N.F.
Filiación:ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, 08860 Castelldefels (Barcelona), Spain
Experimentalphysik IV, Universität Bayreuth, 95440 Bayreuth, Germany
Departamento de Física, Instituto de Física de Buenos Aires (IFIBA, CONICET), Universidad de Buenos Aires, 1438 Buenos Aires, Argentina
ICREA - Institució Catalana de Recerca i Estudis Avançats, 08015 Barcelona, Spain
Palabras clave:Diffraction; Laser beams; Coherent control; Detection volume; Diffraction limits; Orders of magnitude; Pulse stretching; Single molecule; Spatio temporal; Ultrafast pulse; Pulse shaping; nanomaterial; article; chemical model; chemistry; computer simulation; genetic procedures; light; radiation scattering; signal processing; Computer Simulation; Light; Models, Chemical; Molecular Probe Techniques; Nanostructures; Scattering, Radiation; Signal Processing, Computer-Assisted
Año:2011
Volumen:19
Número:27
Página de inicio:26486
Página de fin:26499
DOI: http://dx.doi.org/10.1364/OE.19.026486
Título revista:Optics Express
Título revista abreviado:Opt. Express
ISSN:10944087
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_10944087_v19_n27_p26486_Brinks

Referencias:

  • Meshulach, D., Silberberg, Y., Coherent quantum control of two-photo transitions by a femtosecond laser pulse (1998) Nature, 396 (6708), pp. 239-242. , DOI 10.1038/24329
  • Herek, J.L., Wohlleben, W., Cogdell, R.J., Zeidler, D., Motzkus, M., Quantum control of energy flow in light harvesting (2002) Nature, 417 (6888), pp. 533-535. , DOI 10.1038/417533a
  • Prokhorenko, V.I., Nagy, A.M., Waschuk, S.A., Brown, L.S., Birge, R.R., Miller, R.J.D., Coherent control of retinal isomerization in bacteriorhodopsin (2006) Science, 313 (5791), pp. 1257-1261. , DOI 10.1126/science.1130747
  • Voronine, D.V., Abramavicius, D., Mukamel, S., Coherent control protocol for separating energy-transfer pathways in photosynthetic complexes by chiral multidimensional signals (2011) J. Phys. Chem. A, 115 (18), pp. 4624-4629
  • Assion, A., Baumert, T., Bergt, M., Brixner, T., Kiefer, B., Seyfried, V., Strehle, M., Gerber, G., Control of chemical reactions by feedback-optimized phase-shaped femtosecond laser pulses (1998) Science, 282 (5390), pp. 919-922. , DOI 10.1126/science.282.5390.919
  • Brixner, T., Gerber, G., Quantum control of gas-phase and liquid-phase femtochemistry (2003) ChemPhysChem, 4 (5), pp. 418-438
  • Lozovoy, V.V., Dantus, M., Systematic control of nonlinear optical processes using optimally shaped femtosecond pulses (2005) ChemPhysChem, 6 (10), pp. 1970-2000
  • Stanciu, C.D., Hansteen, F., Kimel, A.V., Kirilyuk, A., Tsukamoto, A., Itoh, A., Rasing, T., All-optical magnetic recording with circularly polarized light (2007) Phys. Rev. Lett., 99 (4), p. 047601
  • Hillerkuss, D., Schmogrow, R., Schellinger, T., Jordan, M., Winter, M., Huber, G., Vallaitis, T., Leuthold, J., 26 Tbit s-1 linerate super-channel transmission utilizing all-optical fast Fourier transform processing (2011) Nat. Photonics, 5 (6), pp. 364-371
  • Jiang, Z., Huang, C.-B., Leaird, D.E., Weiner, A.M., Optical arbitrary waveform processing of more than 100 spectral comb lines (2007) Nat. Photonics, 1 (8), pp. 463-467
  • Král, P., Thanopulos, I., Shapiro, M., Coherently controlled adiabatic passage (2007) Rev. Mod. Phys., 79 (1), pp. 53-77
  • Greentree, A., Devitt, S., Hollenberg, L., Quantum-information transport to multiple receivers (2006) Phys. Rev. A, 73 (3), p. 032319
  • Rabitz, H., De Vivie-Riedle, R., Motzkus, M., Kompa, K., Whither the future of controlling quantum phenomena? (2000) Science, 288 (5467), pp. 824-828. , DOI 10.1126/science.288.5467.824
  • Kuroda, D.G., Singh, C.P., Peng, Z., Kleiman, V.D., Mapping excited-state dynamics by coherent control of a dendrimer's photoemission efficiency (2009) Science, 326 (5950), pp. 263-267
  • Engel, G.S., Calhoun, T.R., Read, E.L., Ahn, T.-K., Mancal, T., Cheng, Y.-C., Blankenship, R.E., Fleming, G.R., Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems (2007) Nature, 446 (7137), pp. 782-786. , DOI 10.1038/nature05678, PII NATURE05678
  • Collini, E., Wong, C.Y., Wilk, K.E., Curmi, P.M.G., Brumer, P., Scholes, G.D., Coherently wired lightharvesting in photosynthetic marine algae at ambient temperature (2010) Nature, 463 (7281), pp. 644-647
  • Brinks, D., Stefani, F.D., Kulzer, F., Hildner, R., Taminiau, T.H., Avlasevich, Y., Müllen, K., Van Hulst, N.F., Visualizing and controlling vibrational wave packets of single molecules (2010) Nature, 465 (7300), pp. 905-908
  • Hildner, R., Brinks, D., Van Hulst, N.F., Femtosecond coherence and quantum control of single molecules at room temperature (2011) Nat. Phys., 7 (2), pp. 172-177
  • Min, W., Lu, S., Chong, S., Roy, R., Holtom, G.R., Xie, X.S., Imaging chromophores with undetectable fluorescence by stimulated emission microscopy (2009) Nature, 461 (7267), pp. 1105-1109
  • Saar, B.G., Freudiger, C.W., Reichman, J., Stanley, C.M., Holtom, G.R., Xie, X.S., Video-rate molecular imaging in vivo with stimulated Raman scattering (2010) Science, 330 (6009), pp. 1368-1370
  • Freudiger, C.W., Min, W., Holtom, G.R., Xu, B., Dantus, M., Sunney Xie, X., Highly specific label-free molecular imaging with spectrally tailored excitation-stimulated Raman scattering (STE-SRS) microscopy (2011) Nat. Photonics, 5 (2), pp. 103-109
  • Zeidler, D., Hornung, T., Proch, D., Motzkus, M., Adaptive compression of tunable pulses from a noncollinear-type OPA to below 16 fs by feedback-controlled pulse shaping (2000) Appl. Phys. B, 131, pp. 125-131
  • Tan, H.-S., Schreiber, E., Warren, W.S., High-resolution indirect pulse shaping by parametric transfer (2002) Optics Letters, 27 (6), pp. 439-441
  • Lorenc, D., Velic, D., Markevitch, A.N., Levis, R.J., Adaptive femtosecond pulse shaping to control supercontinuum generation in a microstructure fiber (2007) Optics Communications, 276 (2), pp. 288-292. , DOI 10.1016/j.optcom.2007.04.015, PII S0030401807004087
  • Ganz, T., Pervak, V., Apolonski, A., Baum, P., 16 fs, 350 nJ pulses at 5 MHz repetition rate delivered by chirped pulse compression in fibers (2011) Opt. Lett., 36 (7), pp. 1107-1109
  • Martinez, O.E., Gordon, J.P., Fork, R.L., Negative group-velocity dispersion using refraction (1984) Journal of the Optical Society of America A: Optics and Image Science, and Vision, 1 (10), pp. 1003-1006
  • Treacy, E., Optical pulse compression with diffraction gratings (1969) IEEE J. Quantum Electron., 5 (9), pp. 454-458
  • Martinez, O., Design of high-power ultrashort pulse amplifiers by expansion and recompression (1987) IEEE Journal of Quantum Electronics, QE-23 (8), pp. 1385-1387
  • Szipocs, R., Ferencz, K., Spielmann, C., Krausz, F., Chirped multilayer coatings for broadband dispersion control in femtosecond lasers (1994) Opt. Lett., 19 (3), pp. 201-203
  • Brixner, T., Gerber, G., Femtosecond polarization pulse shaping (2001) Optics Letters, 26 (8), pp. 557-559
  • Aeschlimann, M., Bauer, M., Bayer, D., Brixner, T., Garcia De Abajo, F.J., Pfeiffer, W., Rohmer, M., Steeb, F., Adaptive subwavelength control of nano-optical fields (2007) Nature, 446 (7133), pp. 301-304. , DOI 10.1038/nature05595, PII NATURE05595
  • Weiner, A.M., Femtosecond pulse shaping using spatial light modulators (2000) Rev. Sci. Instrum., 71 (5), pp. 1929-1960
  • Weiner, A.M., Leaird, D.E., Wiederrecht, G.P., Nelson, K.A., Femtosecond pulse sequences used for optical manipulation of molecular motion (1990) Science, 247 (4948), pp. 1317-1319
  • Weiner, A.M., Leaird, D.E., Patel, J.S., Wullert, J.R., Programmable shaping of femtosecond optical pulses by use of 128-element liquid crystal phase modulator (1992) IEEE J. Quantum Electron., 28 (4), pp. 908-920
  • Weiner, A.M., Leaird, D.E., Patel, J.S., Wullert, J.R., Programmable femtosecond pulse shaping by use of a multielement liquid-crystal phase modulator (1990) Opt. Lett., 15 (6), pp. 326-328
  • Tian, P., Keusters, D., Suzaki, Y., Warren, W.S., Femtosecond phase-coherent two-dimensional spectroscopy (2003) Science, 300 (5625), pp. 1553-1555. , DOI 10.1126/science.1083433
  • Krebs, N., Probst, R.A., Riedle, E., Sub-20 fs pulses shaped directly in the UV by an acousto-optic programmable dispersive filter (2010) Opt. Express, 18 (6), pp. 6164-6171
  • Dixon, R., Acoustic diffraction of light in anisotropic media (1967) IEEE J. Quantum Electron., 3 (2), pp. 85-93
  • Tournois, P., Acousto-optic programmable dispersive filter for adaptive compensation of group delay time dispersion in laser systems (1997) Optics Communications, 140 (4-6), pp. 245-249. , PII S0030401897001533
  • Verluise, F., Laude, V., Cheng, Z., Spielmann, C., Tournois, P., Amplitude and phase control of ultrashort pulses by use of an acousto-optic programmable dispersive filter: Pulse compression and shaping (2000) Opt. Lett., 25 (8), pp. 575-577
  • Verluise, F., Laude, V., Huignard, J.P., Tournois, P., Migus, A., Arbitrary dispersion control of ultrashort optical pulses with acoustic waves (2000) J. Opt. Soc. Am. B, 17 (1), pp. 138-145
  • Dorrer, C., Salin, F., Phase amplitude coupling in spectral phase modulation (1998) IEEE Journal on Selected Topics in Quantum Electronics, 4 (2), pp. 342-345. , PII S1077260X98037630
  • Tanabe, T., Tanabe, H., Teramura, Y., Kannari, F., Spatiotemporal measurements based on spatial spectral interferometry for ultrashort optical pulses shaped by a Fourier pulse shaper (2002) J. Opt. Soc. Am. B, 19 (11), pp. 2795-2802
  • Monmayrant, A., Weber, S., Chatel, B., A newcomer's guide to ultrashort pulse shaping and characterization (2010) J. Phys. At. Mol. Opt. Phys., 43 (10), p. 103001
  • McCabe, D.J., Austin, D.R., Tajalli, A., Weber, S., Walmsley, I.A., Chatel, B., Space-time coupling of shaped ultrafast ultraviolet pulses from an acousto-optic programmable dispersive filter (2011) J. Opt. Soc. Am. B, 28 (1), pp. 58-64
  • Martinez, O.E., Grating and prism compressors in the case of finite beam size (1986) J. Opt. Soc. Am. B, 3 (7), pp. 929-934
  • Bonadeo, N.H., Erland, J., Gammon, D., Park, D., Katzer, D.S., Steel, D.G., Coherent optical control of the quantum state of a single quantum dot (1998) Science, 282 (5393), pp. 1473-1476
  • Brinks, D., Stefani, F.D., Van Hulst, N.F., Nanoscale spatial effects of pulse shaping (2009) Springer Ser. Chem. Phys., 92, pp. 890-892
  • Sussman, B., Lausten, R., Stolow, A., Focusing of light following a 4-f pulse shaper: Considerations for quantum control (2008) Phys. Rev. A, 77 (4), p. 043416
  • Frei, F., Bloch, R., Feurer, T., Influence of finite spatial resolution on single- and double-pass femtosecond pulse shapers (2010) Opt. Lett., 35 (23), pp. 4072-4074
  • Goodman, J.W., (2005) Introduction to Fourier Optics, , 3rd ed. (Roberts & Company Publishers)
  • Wefers, M.M., Nelson, K.A., Space-time profiles of shaped ultrafast optical waveforms (1996) IEEE Journal of Quantum Electronics, 32 (1), pp. 161-172. , PII S0018919796003508
  • Anderson, A., Deryckx, K.S., Xu, X.G., Steinmeyer, G., Raschke, M.B., Few-femtosecond plasmon dephasing of a single metallic nanostructure from optical response function reconstruction by interferometric frequency resolved optical gating (2010) Nano Lett., 10 (7), pp. 2519-2524
  • Sadiq, D., Shirdel, J., Lee, J.S., Selishcheva, E., Park, N., Lienau, C., Adiabatic nanofocusing scattering-type optical nanoscopy of individual gold nanoparticles (2011) Nano Lett., 11 (4), pp. 1609-1613
  • Hildner, R., Brinks, D., Stefani, F.D., Van Hulst, N.F., Electronic coherences and vibrational wave-packets in single molecules studied with femtosecond phase-controlled spectroscopy (2011) Phys. Chem. Chem. Phys., 13 (5), pp. 1888-1894
  • Strickland, D., Mourou, G., Compression of amplified chirped optical pulses (1985) Optics Communications, 56 (3), pp. 219-221. , DOI 10.1016/0030-4018(85)90120-8
  • Wefers, M.M., Nelson, K.A., Analysis of programmable ultrashort waveform generation using liquid-crystal spatial light modulators (1995) J. Opt. Soc. Am. B, 12 (7), pp. 1343-1362
  • Avlasevich, Y., Muller, S., Erk, P., Mullen, K., Novel core-expanded rylenebis(dicarboximide) dyes bearing pentacene units: Facile synthesis and photophysical properties (2007) Chemistry - A European Journal, 13 (23), pp. 6555-6561. , DOI 10.1002/chem.200700523

Citas:

---------- APA ----------
Brinks, D., Hildner, R., Stefani, F.D. & Van Hulst, N.F. (2011) . Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments. Optics Express, 19(27), 26486-26499.
http://dx.doi.org/10.1364/OE.19.026486
---------- CHICAGO ----------
Brinks, D., Hildner, R., Stefani, F.D., Van Hulst, N.F. "Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments" . Optics Express 19, no. 27 (2011) : 26486-26499.
http://dx.doi.org/10.1364/OE.19.026486
---------- MLA ----------
Brinks, D., Hildner, R., Stefani, F.D., Van Hulst, N.F. "Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments" . Optics Express, vol. 19, no. 27, 2011, pp. 26486-26499.
http://dx.doi.org/10.1364/OE.19.026486
---------- VANCOUVER ----------
Brinks, D., Hildner, R., Stefani, F.D., Van Hulst, N.F. Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments. Opt. Express. 2011;19(27):26486-26499.
http://dx.doi.org/10.1364/OE.19.026486