Abstract:
Large-size mesoporous thin films with a mixed titania-silica framework and an Im over(3, -) m cubic-derived or worm-like mesostructure were obtained by combining sol-gel and macromolecular templating techniques. These materials presented accessible mesopores (20 to 25% pore volume), tunable refractive index and high molecular-scale mixing of both ions, as demonstrated by UV-Visible, FTIR and XANES spectroscopy. In addition, a composition effect in the catalytic reduction of silver was found, which permitted one to obtain homogeneous metal nanoparticle-mesoporous film nanocomposites with tuned plasmon position. © 2009 Académie des sciences.
Registro:
Documento: |
Artículo
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Título: | Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks |
Autor: | Angelomé, P.C.; Andrini, L.; Fuertes, M.C.; Requejo, F.G.; Soler-Illia, G.J.A.A. |
Filiación: | Gerencia de Química, CNEA, Centro Atómico Constituyentes, Avenue Gral Paz 1499, San Martín, B1650KNA, Argentina Departamento Física, FCE, UNLP and INIFTA-IFLP (CONICET), CC/67, 1900 La Plata, Argentina CONICET, Avenue Rivadavia 1917, C1033AAJ Buenos Aires, Argentina DQIAyQF, FCEN, Universidad de Buenos Aires, Ciudad Universitaria, Pabellon II, C1428EHA Buenos Aires, Argentina
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Palabras clave: | Catalysis; Mesoporous films; Mixed oxides; Self-assembly; Sol-gel |
Año: | 2010
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Volumen: | 13
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Número: | 1-2
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Página de inicio: | 256
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Página de fin: | 269
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DOI: |
http://dx.doi.org/10.1016/j.crci.2009.07.001 |
Título revista: | Comptes Rendus Chimie
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Título revista abreviado: | C. R. Chim.
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ISSN: | 16310748
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CODEN: | CRCOC
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Registro: | https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_16310748_v13_n1-2_p256_Angelome |
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Citas:
---------- APA ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G. & Soler-Illia, G.J.A.A.
(2010)
. Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks. Comptes Rendus Chimie, 13(1-2), 256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001---------- CHICAGO ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G., Soler-Illia, G.J.A.A.
"Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks"
. Comptes Rendus Chimie 13, no. 1-2
(2010) : 256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001---------- MLA ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G., Soler-Illia, G.J.A.A.
"Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks"
. Comptes Rendus Chimie, vol. 13, no. 1-2, 2010, pp. 256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001---------- VANCOUVER ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G., Soler-Illia, G.J.A.A. Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks. C. R. Chim. 2010;13(1-2):256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001